Vibrational energy transport in the presence of intrasite vibrational energy redistribution
نویسندگان
چکیده
منابع مشابه
Vibrational energy transport in the presence of intrasite vibrational energy redistribution.
The mechanism of vibrational energy flow is studied in a regime where a diffusion equation is likely to break down, i.e., on length scales of a few chemical bonds and time scales of a few picoseconds. This situation occurs, for example, during photochemical reactions in protein environment. To that end, a toy model is introduced that on the one hand mimics the vibrational normal mode distributi...
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ژورنال
عنوان ژورنال: The Journal of Chemical Physics
سال: 2009
ISSN: 0021-9606,1089-7690
DOI: 10.1063/1.3185152